Rod Taylor

as Pongo (voice)

J. Pat O'Malley

as Colonel / Jasper (voice)

Betty Lou Gerson

as Cruella De Vil / Miss Birdwell (voice)

Martha Wentworth

as Nanny / Queenie / Lucy (voice)

Ben Wright

as Roger (voice)

Cate Bauer

as Perdita (voice)

David Frankham

as Sergeant Tibbs (voice)

Frederick Worlock

as Horace / Inspector Craven (voice)